CH4 hydrate dissociation and CH4 leakage characteristics: Insights from laboratory investigation based on stratified environment reconstruction of natural gas hydrate reservoir

Yan Xie, Jing-Chun Feng, Xingyu Chen, Junwen Wang, Longhang Xu, Zhenwu Zhou, Bin Wang, Yi Wang, Si Zhang and Zhifeng Yang

Renewable and Sustainable Energy Reviews, 2024, vol. 206, issue C

Abstract: Submarine natural gas hydrates (NGHs) are one of the largest methane reservoirs on Earth, offering huge potential as an alternative energy source and serving as a crucial global carbon sink. However, the substantial risk of methane leakage during NGH development seriously threatens marine and global ecological and environmental safety, presenting a major challenge for commercial NGH exploitation. Focusing on the unknown leakage mechanisms, this study employed a new simulation device to construct a stratified environment and to investigate the characteristics of hydrate dissociation and methane leakage during depressurization production, under conditions of varied fracturing in overlying sediment. A movable module was used to dynamically isolate and connect the hydrate reservoir with the overlying layer. The results showed that the intrusion of overlying water decelerated the reservoir depressurization rate, leading to a mass of hydrate reformation. The invasion locations and flow paths of the overlying water were influenced by the fracture scale of the overlying sediment. Benefiting from the additional sensible heat and reservoir space occupation of the overlying water in the later production stages, the methane recovery ratio in the fracture-containing systems were not significantly affected. However, the leakage methane increased as fracture channels enlarged, reaching up to 9.90 % of the total methane content in the hydrate reservoir. The leakage mechanism primarily involved local overpressure, buoyancy effects, and diffusion. The research, for the first time, experimentally revealed the response relationship between methane leakage and hydrate dissociation, providing foundational data and theoretical support for the safe and efficient NGH development.

Keywords: CH4 hydrate exploitation; CH4 leakage; Stratified environment; Permeable overburden; Fractures (search for similar items in EconPapers)
Date: 2024
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DOI: 10.1016/j.rser.2024.114891

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