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Insights into Enhancing Electrochemical Performance of Li-Ion Battery Anodes via Polymer Coating

Mozaffar Abdollahifar (), Palanivel Molaiyan, Milena Perovic and Arno Kwade
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Mozaffar Abdollahifar: Institute for Particle Technology, Technische Universität Braunschweig, Volkmaroder Str. 5, 38104 Braunschweig, Germany
Palanivel Molaiyan: Research Unit of Sustainable Chemistry, University of Oulu, 90570 Oulu, Finland
Milena Perovic: Institute for Particle Technology, Technische Universität Braunschweig, Volkmaroder Str. 5, 38104 Braunschweig, Germany
Arno Kwade: Institute for Particle Technology, Technische Universität Braunschweig, Volkmaroder Str. 5, 38104 Braunschweig, Germany

Energies, 2022, vol. 15, issue 23, 1-28

Abstract: Due to the ever-growing importance of rechargeable lithium-ion batteries, the development of electrode materials and their processing techniques remains a hot topic in academia and industry. Even the well-developed and widely utilized active materials present issues, such as surface reactivity, irreversible capacity in the first cycle, and ageing. Thus, there have been many efforts to modify the surface of active materials to enhance the electrochemical performance of the resulting electrodes and cells. Herein, we review the attempts to use polymer coatings on the anode active materials. This type of coating stands out because of the possibility of acting as an artificial solid electrolyte interphase (SEI), serving as an anode protective layer. We discuss the prominent examples of anodes with different mechanisms: intercalation (graphite and titanium oxides), alloy (silicon, tin, and germanium), and conversion (transition metal oxides) anodes. Finally, we give our perspective on the future developments in this field.

Keywords: polymer coating; anode materials; lithium-ion batteries; artificial solid electrolyte interphase (search for similar items in EconPapers)
JEL-codes: Q Q0 Q4 Q40 Q41 Q42 Q43 Q47 Q48 Q49 (search for similar items in EconPapers)
Date: 2022
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