Numerical Analysis of Soot Dynamics in C 3 H 8 Oxy-Combustion with CO 2 and H 2 O

Yue Xin, Bowen Liang, Yindi Zhang (), Mengting Si and Jinisper Joseph Cunatt
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Yue Xin: School of Petroleum Engineering, Yangtze University, Wuhan 430100, China
Bowen Liang: School of Petroleum Engineering, Yangtze University, Wuhan 430100, China
Yindi Zhang: School of Petroleum Engineering, Yangtze University, Wuhan 430100, China
Mengting Si: School of Petroleum Engineering, Yangtze University, Wuhan 430100, China
Jinisper Joseph Cunatt: School of Petroleum Engineering, Yangtze University, Wuhan 430100, China

Energies, 2024, vol. 17, issue 24, 1-32

Abstract: Oxygen-enriched combustion is increasingly recognized as a viable approach for clean energy production and carbon capture, offering substantial benefits for boosting combustion efficiency and mitigating pollutant emissions, which makes it widely adopted in various industrial applications. Liquefied petroleum gas (LPG), predominantly consisting of propane (C 3 H 8 ), is commonly utilized in numerous combustion systems, yet its emissions of soot particulates have raised considerable environmental concerns. This study delves into the combustion dynamics and soot formation behavior of propane, the principal component of LPG, under oxy-fuel combustion conditions, with the inclusion of H 2 O and CO 2 , utilizing both experimental techniques and numerical simulations. The results reveal that CO 2 and H 2 O suppress soot formation through distinct mechanisms. CO 2 decreases soot nucleation and surface growth by lowering flame temperature and H atom concentration, but it minimally enhances soot oxidation. H 2 O significantly reduces soot formation by chemically increasing OH radical concentration, thereby enhancing soot oxidation. A detailed decoupling analysis further shows that CO 2 ’s influence is predominantly thermal and chemical, resulting in lower OH levels and an elongated flame shape. In contrast, H 2 O’s substantial thermal and chemical effects decrease flame height and promote soot reduction. These insights advance the understanding of soot formation control in oxy-fuel combustion, offering strategies to optimize combustion efficiency and minimize environmental impact.

Keywords: oxy-combustion; CO 2 /C 3 H 8; soot formation; combustion modeling; hydrocarbon fuels (search for similar items in EconPapers)
JEL-codes: Q Q0 Q4 Q40 Q41 Q42 Q43 Q47 Q48 Q49 (search for similar items in EconPapers)
Date: 2024
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