Polycycl. Aromatic Hydrocarbon Exposure of Children in Typical Household Coal Combustion Environments: Seasonal Variations, Sources, and Carcinogenic Risks

Yunwei Liu, Ning Qin, Weigang Liang, Xing Chen, Rong Hou, Yijin Kang, Qian Guo, Suzhen Cao and Xiaoli Duan
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Yunwei Liu: School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, China
Ning Qin: School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, China
Weigang Liang: School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, China
Xing Chen: School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, China
Rong Hou: School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, China
Yijin Kang: School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, China
Qian Guo: School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, China
Suzhen Cao: School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, China
Xiaoli Duan: School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, China

IJERPH, 2020, vol. 17, issue 18, 1-14

Abstract: Polycyclic aromatic hydrocarbon (PAH) emissions from the combustion of household solid coal for cooking and heating cause great harm to public health in China, especially in less developed areas. Children are one of the most susceptible population groups at risk of indoor air pollutants due to their immature respiratory and immune systems. However, information on PAH exposure of children is limited due to limited monitoring data. In this study, we aimed to assess the seasonal differences of PAHs in classrooms, analyze the pollutant sources, and calculate the incremental lifetime cancer risk attributable to PAHs in Shanxi Provence. A typical school using household coal combustion in Shanxi Province was selected. Fine particulate matter (PM 2.5 )samples were collected by both individual samplers and fixed middle-flow samplers during the heating and non-heating seasons in December 2018 and April 2019. The PAH concentrations in PM 2.5 samples were analyzed by a gas chromatograph coupled to a mass spectrometer. The results showed that PAH concentrations in PM 2.5 varied between 89.1 ng/m 3 in the heating season and 1.75 ng/m 3 in the non-heating season. The mean concentrations of benzo[a]pyrene (BaP), a carcinogenic marker of PAHs, were 10.3 and 0.05 ng/m 3 in the heating and non-heating seasons, respectively. Source allocation analysis of individual portable and passive samplers revealed that the main contributors during heating and non-heating seasons were coal combustion and gasoline sources, respectively. According to the results of a Monte Carlo simulation, the incremental lifetime cancer risk values from the inhalation of PAHs in the heating and non-heating seasons were 3.1 × 10 −6 and 5.7 × 10 −8 , respectively. The significant increase in PAHs and the incremental lifetime cancer risk in the heating season indicates that children are more exposed to health threats in winter. Further PAH exposure control strategies, including reducing coal usage and promoting clean fuel applications, need to be developed to reduce the risk of PAH-induced cancer.

Keywords: seasonal variation; children exposure; household solid fuel; polycyclic aromatic hydrocarbons; risk assessment (search for similar items in EconPapers)
JEL-codes: I I1 I3 Q Q5 (search for similar items in EconPapers)
Date: 2020
References: View references in EconPapers View complete reference list from CitEc
Citations: View citations in EconPapers (4)

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