A Review on N-Doped Biochar for Oxidative Degradation of Organic Contaminants in Wastewater by Persulfate Activation

Yaxuan Gao, Wenran Gao, Haonan Zhu, Haoran Chen, Shanshan Yan, Ming Zhao, Hongqi Sun, Junjie Zhang and Shu Zhang ()
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Yaxuan Gao: Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, Joint International Research Laboratory of Biomass Energy and Materials, College of Materials Science and Engineering, Nanjing Forestry University, Nanjing 210037, China
Wenran Gao: Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, Joint International Research Laboratory of Biomass Energy and Materials, College of Materials Science and Engineering, Nanjing Forestry University, Nanjing 210037, China
Haonan Zhu: Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, Joint International Research Laboratory of Biomass Energy and Materials, College of Materials Science and Engineering, Nanjing Forestry University, Nanjing 210037, China
Haoran Chen: Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, Joint International Research Laboratory of Biomass Energy and Materials, College of Materials Science and Engineering, Nanjing Forestry University, Nanjing 210037, China
Shanshan Yan: Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, Joint International Research Laboratory of Biomass Energy and Materials, College of Materials Science and Engineering, Nanjing Forestry University, Nanjing 210037, China
Ming Zhao: Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, Joint International Research Laboratory of Biomass Energy and Materials, College of Materials Science and Engineering, Nanjing Forestry University, Nanjing 210037, China
Hongqi Sun: School of Engineering, Edith Cowan University, Joondalup, WA 6027, Australia
Junjie Zhang: State Key Laboratory of Organic Electronics and Information Displays, Institute of Advanced Materials, School of Material Science and Engineering, Nanjing University of Posts and Telecommunications, Nanjing 210023, China
Shu Zhang: Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, Joint International Research Laboratory of Biomass Energy and Materials, College of Materials Science and Engineering, Nanjing Forestry University, Nanjing 210037, China

IJERPH, 2022, vol. 19, issue 22, 1-25

Abstract: The Persulfate-based advanced oxidation process is the most efficient and commonly used technology to remove organic contaminants in wastewater. Due to the large surface area, unique electronic properties, abundant N functional groups, cost-effectiveness, and environmental friendliness, N-doped biochars (NBCs) are widely used as catalysts for persulfate activation. This review focuses on the NBC for oxidative degradation of organics-contaminated wastewater. Firstly, the preparation and modification methods of NBCs were reviewed. Then the catalytic performance of NBCs and modified NBCs on the oxidation degradation of organic contaminants were discussed with an emphasis on the degradation mechanism. We further summarized the detection technologies of activation mechanisms and the structures of NBCs affecting the PS activation, followed by the specific role of the N configuration of the NBC on its catalytic capacity. Finally, several challenges in the treatment of organics-contaminated wastewater by a persulfate-based advanced oxidation process were put forward and the recommendations for future research were proposed for further understanding of the advanced oxidation process activated by the NBC.

Keywords: N-doped biochar; persulfate; advanced oxidation process; N configuration; wastewater (search for similar items in EconPapers)
JEL-codes: I I1 I3 Q Q5 (search for similar items in EconPapers)
Date: 2022
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