Nanoprinting organic molecules at the quantum level

Claudio U. Hail, Christian Höller, Korenobu Matsuzaki, Patrik Rohner, Jan Renger, Vahid Sandoghdar, Dimos Poulikakos () and Hadi Eghlidi ()
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Claudio U. Hail: ETH Zürich
Christian Höller: ETH Zürich
Korenobu Matsuzaki: Max Planck Institute for the Science of Light
Patrik Rohner: ETH Zürich
Jan Renger: Max Planck Institute for the Science of Light
Vahid Sandoghdar: Max Planck Institute for the Science of Light
Dimos Poulikakos: ETH Zürich
Hadi Eghlidi: ETH Zürich

Nature Communications, 2019, vol. 10, issue 1, 1-8

Abstract: Abstract Organic compounds present a powerful platform for nanotechnological applications. In particular, molecules suitable for optical functionalities such as single photon generation and energy transfer have great promise for complex nanophotonic circuitry due to their large variety of spectral properties, efficient absorption and emission, and ease of synthesis. Optimal integration, however, calls for control over position and orientation of individual molecules. While various methods have been explored for reaching this regime in the past, none satisfies requirements necessary for practical applications. Here, we present direct non-contact electrohydrodynamic nanoprinting of a countable number of photostable and oriented molecules in a nanocrystal host with subwavelength positioning accuracy. We demonstrate the power of our approach by writing arbitrary patterns and controlled coupling of single molecules to the near field of optical nanostructures. Placement precision, high yield and fabrication facility of our method open many doors for the realization of novel nanophotonic devices.

Date: 2019
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DOI: 10.1038/s41467-019-09877-5

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