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Controllable two-dimensional movement and redistribution of lithium ions in metal oxides

Xiufeng Tang, Guoxin Chen, Zhaopeng Mo, Dingbang Ma, Siyuan Wang, Jinxiu Wen, Li Gong, Lite Zhao, Jingcheng Huang, Tengcheng Huang and Jianyi Luo ()
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Xiufeng Tang: Wuyi University
Guoxin Chen: Wuyi University
Zhaopeng Mo: Wuyi University
Dingbang Ma: Wuyi University
Siyuan Wang: Wuyi University
Jinxiu Wen: Wuyi University
Li Gong: Sun Yat-sen University
Lite Zhao: Wuyi University
Jingcheng Huang: Wuyi University
Tengcheng Huang: Wuyi University
Jianyi Luo: Wuyi University

Nature Communications, 2019, vol. 10, issue 1, 1-7

Abstract: Abstract Rechargeable lithium batteries are the most practical and widely used power sources for portable and mobile devices in modern society. Manipulation of the electronic and ionic charge transport and accumulation in solid materials has always been crucial for rechargeable lithium batteries. The transport and accumulation of lithium ions in electrode materials, which is a diffusion process, is determined by the concentration distribution of lithium ions and the intrinsic structure of the electrode material and thus far has not been manipulated by an external force. Here, we report the realization of controllable two-dimensional movement and redistribution of lithium ions in metal oxides. This achievement is one kind of centimeter-scale control and is achieved by a magnetic field based on the ‘current-driving model’. This work provides additional insight for building safe and high-capacity rechargeable lithium batteries.

Date: 2019
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DOI: 10.1038/s41467-019-10875-w

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