Optically pumped colloidal-quantum-dot lasing in LED-like devices with an integrated optical cavity
Jeongkyun Roh,
Young-Shin Park,
Jaehoon Lim and
Victor I. Klimov ()
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Jeongkyun Roh: Los Alamos National Laboratory
Young-Shin Park: Los Alamos National Laboratory
Jaehoon Lim: Los Alamos National Laboratory
Victor I. Klimov: Los Alamos National Laboratory
Nature Communications, 2020, vol. 11, issue 1, 1-10
Abstract:
Abstract Realization of electrically pumped lasing with solution processable materials will have a revolutionary impact on many disciplines including photonics, chemical sensing, and medical diagnostics. Due to readily tunable, size-controlled emission wavelengths, colloidal semiconductor quantum dots (QDs) are attractive materials for attaining this goal. Here we use specially engineered QDs to demonstrate devices that operate as both a light emitting diode (LED) and an optically pumped laser. These structures feature a distributed feedback resonator integrated into a bottom LED electrode. By carefully engineering a refractive-index profile across the device, we are able to obtain good confinement of a waveguided mode within the QD medium, which allows for demonstrating low-threshold lasing even with an ultrathin (about three QD monolayers) active layer. These devices also exhibit strong electroluminescence (EL) under electrical pumping. The conducted studies suggest that the demonstrated dual-function (lasing/EL) structures represent a promising device platform for realizing colloidal QD laser diodes.
Date: 2020
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Persistent link: https://EconPapers.repec.org/RePEc:nat:natcom:v:11:y:2020:i:1:d:10.1038_s41467-019-14014-3
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DOI: 10.1038/s41467-019-14014-3
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