Emergent solidity of amorphous materials as a consequence of mechanical self-organisation

Hua Tong, Shiladitya Sengupta and Hajime Tanaka ()
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Hua Tong: Shanghai Jiao Tong University
Shiladitya Sengupta: University of Tokyo
Hajime Tanaka: University of Tokyo

Nature Communications, 2020, vol. 11, issue 1, 1-10

Abstract: Abstract Amorphous solids have peculiar properties distinct from crystals. One of the most fundamental mysteries is the emergence of solidity in such nonequilibrium, disordered state without the protection by long-range translational order. A jammed system at zero temperature, although marginally stable, has solidity stemming from the space-spanning force network, which gives rise to the long-range stress correlation. Here, we show that such nonlocal correlation already appears at the nonequilibrium glass transition upon cooling. This is surprising since we also find that the system suffers from giant anharmonic fluctuations originated from the fractal-like potential energy landscape. We reveal that it is the percolation of the force-bearing network that allows long-range stress transmission even under such circumstance. Thus, the emergent solidity of amorphous materials is a consequence of nontrivial self-organisation of the disordered mechanical architecture. Our findings point to the significance of understanding amorphous solids and nonequilibrium glass transition from a mechanical perspective.

Date: 2020
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DOI: 10.1038/s41467-020-18663-7

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