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Lithography-free IR polarization converters via orthogonal in-plane phonons in α-MoO3 flakes

Sina Abedini Dereshgi, Thomas G. Folland, Akshay A. Murthy, Xianglian Song, Ibrahim Tanriover, Vinayak P. Dravid, Joshua D. Caldwell and Koray Aydin ()
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Sina Abedini Dereshgi: Northwestern University
Thomas G. Folland: Vanderbilt University
Akshay A. Murthy: Northwestern University
Xianglian Song: Northwestern University
Ibrahim Tanriover: Northwestern University
Vinayak P. Dravid: Northwestern University
Joshua D. Caldwell: Vanderbilt University
Koray Aydin: Northwestern University

Nature Communications, 2020, vol. 11, issue 1, 1-9

Abstract: Abstract Exploiting polaritons in natural vdW materials has been successful in achieving extreme light confinement and low-loss optical devices and enabling simplified device integration. Recently, α-MoO3 has been reported as a semiconducting biaxial vdW material capable of sustaining naturally orthogonal in-plane phonon polariton modes in IR. In this study, we investigate the polarization-dependent optical characteristics of cavities formed using α-MoO3 to extend the degrees of freedom in the design of IR photonic components exploiting the in-plane anisotropy of this material. Polarization-dependent absorption over 80% in a multilayer Fabry-Perot structure with α-MoO3 is reported without the need for nanoscale fabrication on the α-MoO3. We observe coupling between the α-MoO3 optical phonons and the Fabry-Perot cavity resonances. Using cross-polarized reflectance spectroscopy we show that the strong birefringence results in 15% of the total power converted into the orthogonal polarization with respect to incident wave. These findings can open new avenues in the quest for polarization filters and low-loss, integrated planar IR photonics and in dictating polarization control.

Date: 2020
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DOI: 10.1038/s41467-020-19499-x

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