Inhomogeneous Kondo-lattice in geometrically frustrated Pr2Ir2O7

Mariam Kavai, Joel Friedman, Kyle Sherman, Mingda Gong, Ioannis Giannakis, Samad Hajinazar, Haoyu Hu, Sarah E. Grefe, Justin Leshen, Qiu Yang, Satoru Nakatsuji, Aleksey N. Kolmogorov, Qimiao Si, Michael Lawler and Pegor Aynajian ()
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Mariam Kavai: Binghamton University
Joel Friedman: Binghamton University
Kyle Sherman: Binghamton University
Mingda Gong: Binghamton University
Ioannis Giannakis: Binghamton University
Samad Hajinazar: Binghamton University
Haoyu Hu: Rice University
Sarah E. Grefe: Rice University
Justin Leshen: Binghamton University
Qiu Yang: University of Tokyo
Satoru Nakatsuji: University of Tokyo
Aleksey N. Kolmogorov: Binghamton University
Qimiao Si: Rice University
Michael Lawler: Binghamton University
Pegor Aynajian: Binghamton University

Nature Communications, 2021, vol. 12, issue 1, 1-8

Abstract: Abstract Magnetic fluctuations induced by geometric frustration of local Ir-spins disturb the formation of long-range magnetic order in the family of pyrochlore iridates. As a consequence, Pr2Ir2O7 lies at a tuning-free antiferromagnetic-to-paramagnetic quantum critical point and exhibits an array of complex phenomena including the Kondo effect, biquadratic band structure, and metallic spin liquid. Using spectroscopic imaging with the scanning tunneling microscope, complemented with machine learning, density functional theory and theoretical modeling, we probe the local electronic states in Pr2Ir2O7 and find an electronic phase separation. Nanoscale regions with a well-defined Kondo resonance are interweaved with a non-magnetic metallic phase with Kondo-destruction. These spatial nanoscale patterns display a fractal geometry with power-law behavior extended over two decades, consistent with being in proximity to a critical point. Our discovery reveals a nanoscale tuning route, viz. using a spatial variation of the electronic potential as a means of adjusting the balance between Kondo entanglement and geometric frustration.

Date: 2021
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DOI: 10.1038/s41467-021-21698-z

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