Highly-efficient electrically-driven localized surface plasmon source enabled by resonant inelastic electron tunneling
Haoliang Qian,
Shilong Li,
Su-Wen Hsu,
Ching-Fu Chen,
Fanglin Tian,
Andrea R. Tao and
Zhaowei Liu ()
Additional contact information
Haoliang Qian: University of California, San Diego, 9500 Gilman Dr
Shilong Li: University of California, San Diego, 9500 Gilman Dr
Su-Wen Hsu: University of California, San Diego, 9500 Gilman Dr
Ching-Fu Chen: University of California, San Diego, 9500 Gilman Dr
Fanglin Tian: University of California, San Diego, 9500 Gilman Dr
Andrea R. Tao: University of California, San Diego, 9500 Gilman Dr
Zhaowei Liu: University of California, San Diego, 9500 Gilman Dr
Nature Communications, 2021, vol. 12, issue 1, 1-7
Abstract:
Abstract On-chip plasmonic circuitry offers a promising route to meet the ever-increasing requirement for device density and data bandwidth in information processing. As the key building block, electrically-driven nanoscale plasmonic sources such as nanoLEDs, nanolasers, and nanojunctions have attracted intense interest in recent years. Among them, surface plasmon (SP) sources based on inelastic electron tunneling (IET) have been demonstrated as an appealing candidate owing to the ultrafast quantum-mechanical tunneling response and great tunability. However, the major barrier to the demonstrated IET-based SP sources is their low SP excitation efficiency due to the fact that elastic tunneling of electrons is much more efficient than inelastic tunneling. Here, we remove this barrier by introducing resonant inelastic electron tunneling (RIET)—follow a recent theoretical proposal—at the visible/near-infrared (NIR) frequencies and demonstrate highly-efficient electrically-driven SP sources. In our system, RIET is supported by a TiN/Al2O3 metallic quantum well (MQW) heterostructure, while monocrystalline silver nanorods (AgNRs) were used for the SP generation (localized surface plasmons (LSPs)). In principle, this RIET approach can push the external quantum efficiency (EQE) close to unity, opening up a new era of SP sources for not only high-performance plasmonic circuitry, but also advanced optical sensing applications.
Date: 2021
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Persistent link: https://EconPapers.repec.org/RePEc:nat:natcom:v:12:y:2021:i:1:d:10.1038_s41467-021-23512-2
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DOI: 10.1038/s41467-021-23512-2
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