Pure spin photocurrent in non-centrosymmetric crystals: bulk spin photovoltaic effect

Haowei Xu, Hua Wang, Jian Zhou and Ju Li ()
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Haowei Xu: Massachusetts Institute of Technology
Hua Wang: Massachusetts Institute of Technology
Jian Zhou: Massachusetts Institute of Technology
Ju Li: Massachusetts Institute of Technology

Nature Communications, 2021, vol. 12, issue 1, 1-9

Abstract: Abstract Spin current generators are critical components for spintronics-based information processing. In this work, we theoretically and computationally investigate the bulk spin photovoltaic (BSPV) effect for creating DC spin current under light illumination. The only requirement for BSPV is inversion symmetry breaking, thus it applies to a broad range of materials and can be readily integrated with existing semiconductor technologies. The BSPV effect is a cousin of the bulk photovoltaic (BPV) effect, whereby a DC charge current is generated under light. Thanks to the different selection rules on spin and charge currents, a pure spin current can be realized if the system possesses mirror symmetry or inversion-mirror symmetry. The mechanism of BSPV and the role of the electronic relaxation time $$\tau$$ τ are also elucidated. We apply our theory to several distinct materials, including monolayer transition metal dichalcogenides, anti-ferromagnetic bilayer MnBi2Te4, and the surface of topological crystalline insulator cubic SnTe.

Date: 2021
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DOI: 10.1038/s41467-021-24541-7

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