Giant room temperature electrocaloric effect in a layered hybrid perovskite ferroelectric: [(CH3)2CHCH2NH3]2PbCl4
Xitao Liu (),
Zhenyue Wu,
Tong Guan,
Haidong Jiang,
Peiqing Long,
Xiaoqi Li,
Chengmin Ji,
Shuang Chen (),
Zhihua Sun and
Junhua Luo ()
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Xitao Liu: Chinese Academy of Sciences
Zhenyue Wu: Chinese Academy of Sciences
Tong Guan: Nanjing University
Haidong Jiang: Nanjing University
Peiqing Long: Chinese Academy of Sciences
Xiaoqi Li: Chinese Academy of Sciences
Chengmin Ji: Chinese Academy of Sciences
Shuang Chen: Nanjing University
Zhihua Sun: Chinese Academy of Sciences
Junhua Luo: Chinese Academy of Sciences
Nature Communications, 2021, vol. 12, issue 1, 1-7
Abstract:
Abstract Electrocaloric effect driven by electric fields displays great potential in realizing highly efficient solid-state refrigeration. Nevertheless, most known electrocaloric materials exhibit relatively poor cooling performance near room temperature, which hinders their further applications. The emerging family of hybrid perovskite ferroelectrics, which exhibits superior structural diversity, large heat exchange and broad property tenability, offers an ideal platform. Herein, we report an exceptionally large electrocaloric effect near room temperature in a designed hybrid perovskite ferroelectric [(CH3)2CHCH2NH3]2PbCl4, which exhibits a sharp first-order phase transition at 302 K, superior spontaneous polarization (>4.8 μC/cm2) and relatively small coercive field (
Date: 2021
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DOI: 10.1038/s41467-021-25644-x
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