Self-healing oxygen evolution catalysts

Agnes E. Thorarinsdottir, Samuel S. Veroneau and Daniel G. Nocera ()
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Agnes E. Thorarinsdottir: Harvard University
Samuel S. Veroneau: Harvard University
Daniel G. Nocera: Harvard University

Nature Communications, 2022, vol. 13, issue 1, 1-10

Abstract: Abstract Electrochemical and photoelectrochemical water splitting offers a scalable approach to producing hydrogen from renewable sources for sustainable energy storage. Depending on the applications, oxygen evolution catalysts (OECs) may perform water splitting under a variety of conditions. However, low stability and/or activity present challenges to the design of OECs, prompting the design of self-healing OECs composed of earth-abundant first-row transition metal oxides. The concept of self-healing catalysis offers a new tool to be employed in the design of stable and functionally active OECs under operating conditions ranging from acidic to basic solutions and from a variety of water sources.

Date: 2022
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DOI: 10.1038/s41467-022-28723-9

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