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A medium-entropy transition metal oxide cathode for high-capacity lithium metal batteries

Yi Pei, Qing Chen, Meiyu Wang, Pengjun Zhang, Qingyong Ren, Jingkai Qin, Penghao Xiao, Li Song, Yu Chen, Wen Yin, Xin Tong, Liang Zhen (), Peng Wang () and Cheng-Yan Xu ()
Additional contact information
Yi Pei: Harbin Institute of Technology (Shenzhen)
Qing Chen: Harbin Institute of Technology (Shenzhen)
Meiyu Wang: Nanjing University
Pengjun Zhang: University of Science and Technology of China
Qingyong Ren: Chinese Academy of Sciences
Jingkai Qin: Harbin Institute of Technology (Shenzhen)
Penghao Xiao: Dalhousie University
Li Song: University of Science and Technology of China
Yu Chen: Chinese Academy of Sciences
Wen Yin: Chinese Academy of Sciences
Xin Tong: Chinese Academy of Sciences
Liang Zhen: Harbin Institute of Technology (Shenzhen)
Peng Wang: Nanjing University
Cheng-Yan Xu: Harbin Institute of Technology (Shenzhen)

Nature Communications, 2022, vol. 13, issue 1, 1-13

Abstract: Abstract The limited capacity of the positive electrode active material in non-aqueous rechargeable lithium-based batteries acts as a stumbling block for developing high-energy storage devices. Although lithium transition metal oxides are high-capacity electrochemical active materials, the structural instability at high cell voltages (e.g., >4.3 V) detrimentally affects the battery performance. Here, to circumvent this issue, we propose a Li1.46Ni0.32Mn1.2O4-x (0

Date: 2022
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DOI: 10.1038/s41467-022-33927-0

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