Spray-coated perovskite hemispherical photodetector featuring narrow-band and wide-angle imaging
Xiaopeng Feng,
Yuhong He,
Wei Qu,
Jinmei Song,
Wanting Pan,
Mingrui Tan,
Bai Yang and
Haotong Wei ()
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Xiaopeng Feng: Jilin University
Yuhong He: Jilin University
Wei Qu: Jilin University
Jinmei Song: Jilin University
Wanting Pan: Jilin University
Mingrui Tan: Jilin University
Bai Yang: Jilin University
Haotong Wei: Jilin University
Nature Communications, 2022, vol. 13, issue 1, 1-9
Abstract:
Abstract Sphere imagers featuring specific wavelength recognition and wide-angle imaging are required to meet the fast development of modern technology. However, it is still challenging to deposit high-quality photosensitive layers on sphere substrates from low-cost solution processes. Here we report spray-coated quasi-two-dimensional phenylethylammonium/formamidinium lead halide (PEA2FAn-1PbnX3n+1) perovskite hemispherical photodetectors. The crystallization speed is manipulated by perovskite compositions, and the film thickness can be controlled by spray-coating cycles and solution concentration from tens of nanometers to hundreds of micrometers with a fast velocity of 1.28 × 10−4 cm3 s−1. The lens-free hemispherical photodetectors allow light response at a wide incident angle of 180°. Simultaneously, the wavelength selective response from visible to the near-infrared range is achieved with full width at half maximums (FWHMs) of ~20 nm, comparable to single-crystal devices. Wide-angle and wavelength-selective imaging are also demonstrated, which can find potential applications in intelligent recognition and intraoperative navigated surgery.
Date: 2022
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Persistent link: https://EconPapers.repec.org/RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-33934-1
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DOI: 10.1038/s41467-022-33934-1
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