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Emergence of electric-field-tunable interfacial ferromagnetism in 2D antiferromagnet heterostructures

Guanghui Cheng, Mohammad Mushfiqur Rahman, Zhiping He, Andres Llacsahuanga Allcca, Avinash Rustagi, Kirstine Aggerbeck Stampe, Yanglin Zhu, Shaohua Yan, Shangjie Tian, Zhiqiang Mao, Hechang Lei, Kenji Watanabe, Takashi Taniguchi, Pramey Upadhyaya and Yong P. Chen ()
Additional contact information
Guanghui Cheng: Tohoku University
Mohammad Mushfiqur Rahman: Purdue University
Zhiping He: University of Science and Technology of China
Andres Llacsahuanga Allcca: Purdue University
Avinash Rustagi: Purdue University
Kirstine Aggerbeck Stampe: Aarhus University
Yanglin Zhu: Pennsylvania State University
Shaohua Yan: Renmin University of China
Shangjie Tian: Renmin University of China
Zhiqiang Mao: Pennsylvania State University
Hechang Lei: Renmin University of China
Kenji Watanabe: National Institute for Materials Science
Takashi Taniguchi: National Institute for Materials Science
Pramey Upadhyaya: Purdue University
Yong P. Chen: Tohoku University

Nature Communications, 2022, vol. 13, issue 1, 1-6

Abstract: Abstract Van der Waals (vdW) magnet heterostructures have emerged as new platforms to explore exotic magnetic orders and quantum phenomena. Here, we study heterostructures of layered antiferromagnets, CrI3 and CrCl3, with perpendicular and in-plane magnetic anisotropy, respectively. Using magneto-optical Kerr effect microscopy, we demonstrate out-of-plane magnetic order in the CrCl3 layer proximal to CrI3, with ferromagnetic interfacial coupling between the two. Such an interlayer exchange field leads to higher critical temperature than that of either CrI3 or CrCl3 alone. We further demonstrate significant electric-field control of the coercivity, attributed to the naturally broken structural inversion symmetry of the heterostructure allowing unprecedented direct coupling between electric field and interfacial magnetism. These findings illustrate the opportunity to explore exotic magnetic phases and engineer spintronic devices in vdW heterostructures.

Date: 2022
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DOI: 10.1038/s41467-022-34812-6

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