Unlocking full and fast conversion in photocatalytic carbon dioxide reduction for applications in radio-carbonylation

Serena Monticelli, Alex Talbot, Philipp Gotico, Fabien Caillé, Olivier Loreau, Antonio Vecchio, Augustin Malandain, Antoine Sallustrau, Winfried Leibl, Ally Aukauloo, Frédéric Taran, Zakaria Halime () and Davide Audisio ()
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Serena Monticelli: Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS
Alex Talbot: Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS
Philipp Gotico: Université Paris-Saclay, CEA, CNRS, Institute for Integrative Biology of the Cell
Fabien Caillé: Université Paris-Saclay, Inserm, CNRS, CEA, Laboratoire d’Imagerie Biomédicale Multimodale Paris-Saclay (BioMaps)
Olivier Loreau: Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS
Antonio Vecchio: Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS
Augustin Malandain: Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS
Antoine Sallustrau: Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS
Winfried Leibl: Université Paris-Saclay, CEA, CNRS, Institute for Integrative Biology of the Cell
Ally Aukauloo: Université Paris-Saclay, CEA, CNRS, Institute for Integrative Biology of the Cell
Frédéric Taran: Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS
Zakaria Halime: Université Paris-Saclay, CNRS, Institut de chimie moléculaire et des matériaux d’Orsay
Davide Audisio: Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS

Nature Communications, 2023, vol. 14, issue 1, 1-10

Abstract: Abstract Harvesting sunlight to drive carbon dioxide (CO2) valorisation represents an ideal concept to support a sustainable and carbon-neutral economy. While the photochemical reduction of CO2 to carbon monoxide (CO) has emerged as a hot research topic, the full CO2-to-CO conversion remains an often-overlooked criterion that prevents a productive and direct valorisation of CO into high-value-added chemicals. Herein, we report a photocatalytic process that unlocks full and fast CO2-to-CO conversion (

Date: 2023
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DOI: 10.1038/s41467-023-40136-w

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