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Synergistic correlated states and nontrivial topology in coupled graphene-insulator heterostructures

Xin Lu, Shihao Zhang, Yaning Wang, Xiang Gao, Kaining Yang, Zhongqing Guo, Yuchen Gao, Yu Ye, Zheng Han and Jianpeng Liu ()
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Xin Lu: ShanghaiTech University
Shihao Zhang: ShanghaiTech University
Yaning Wang: Chinese Academy of Sciences
Xiang Gao: Shanxi University
Kaining Yang: Shanxi University
Zhongqing Guo: ShanghaiTech University
Yuchen Gao: Collaborative Innovation Center of Quantum Matter
Yu Ye: Collaborative Innovation Center of Quantum Matter
Zheng Han: Shanxi University
Jianpeng Liu: ShanghaiTech University

Nature Communications, 2023, vol. 14, issue 1, 1-12

Abstract: Abstract Graphene has aroused great attention due to the intriguing properties associated with its low-energy Dirac Hamiltonian. When graphene is coupled with a correlated insulating substrate, electronic states that cannot be revealed in either individual layer may emerge in a synergistic manner. Here, we theoretically study the correlated and topological states in Coulomb-coupled and gate-tunable graphene-insulator heterostructures. By electrostatically aligning the electronic bands, charge carriers transferred between graphene and the insulator can yield a long-wavelength electronic crystal at the interface, exerting a superlattice Coulomb potential on graphene and generating topologically nontrivial subbands. This coupling can further boost electron-electron interaction effects in graphene, leading to a spontaneous bandgap formation at the Dirac point and interaction-enhanced Fermi velocity. Reciprocally, the electronic crystal at the interface is substantially stabilized with the help of cooperative interlayer Coulomb coupling. We propose a number of substrate candidates for graphene to experimentally demonstrate these effects.

Date: 2023
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DOI: 10.1038/s41467-023-41293-8

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