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Macroscopic tunneling probe of Moiré spin textures in twisted CrI3

Bowen Yang, Tarun Patel, Meixin Cheng, Kostyantyn Pichugin, Lin Tian, Nachiket Sherlekar, Shaohua Yan, Yang Fu, Shangjie Tian, Hechang Lei, Michael E. Reimer, Junichi Okamoto and Adam W. Tsen ()
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Bowen Yang: University of Waterloo
Tarun Patel: University of Waterloo
Meixin Cheng: University of Waterloo
Kostyantyn Pichugin: University of Waterloo
Lin Tian: University of Waterloo
Nachiket Sherlekar: University of Waterloo
Shaohua Yan: Renmin University of China
Yang Fu: Renmin University of China
Shangjie Tian: Renmin University of China
Hechang Lei: Renmin University of China
Michael E. Reimer: University of Waterloo
Junichi Okamoto: University of Freiburg
Adam W. Tsen: University of Waterloo

Nature Communications, 2024, vol. 15, issue 1, 1-8

Abstract: Abstract Various noncollinear spin textures and magnetic phases have been predicted in twisted two-dimensional CrI3 due to competing ferromagnetic (FM) and antiferromagnetic (AFM) interlayer exchange from moiré stacking—with potential spintronic applications even when the underlying material possesses a negligible Dzyaloshinskii–Moriya or dipole–dipole interaction. Recent measurements have shown evidence of coexisting FM and AFM layer order in small-twist-angle CrI3 bilayers and double bilayers. Yet, the nature of the magnetic textures remains unresolved and possibilities for their manipulation and electrical readout are unexplored. Here, we use tunneling magnetoresistance to investigate the collective spin states of twisted double-bilayer CrI3 under both out-of-plane and in-plane magnetic fields together with detailed micromagnetic simulations of domain dynamics based on magnetic circular dichroism. Our results capture hysteretic and anisotropic field evolutions of the magnetic states and we further uncover two distinct non-volatile spin textures (out-of-plane and in-plane domains) at ≈1° twist angle, with a different global tunneling resistance that can be switched by magnetic field.

Date: 2024
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DOI: 10.1038/s41467-024-49261-6

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