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Magnon-phonon Fermi resonance in antiferromagnetic CoF2

Thomas W. J. Metzger (), Kirill A. Grishunin, Chris Reinhoffer, Roman M. Dubrovin, Atiqa Arshad, Igor Ilyakov, Thales V. A. G. Oliveira, Alexey Ponomaryov, Jan-Christoph Deinert, Sergey Kovalev, Roman V. Pisarev, Mikhail I. Katsnelson, Boris A. Ivanov, Paul H. M. Loosdrecht, Alexey V. Kimel and Evgeny A. Mashkovich ()
Additional contact information
Thomas W. J. Metzger: Radboud University
Kirill A. Grishunin: Radboud University
Chris Reinhoffer: University of Cologne
Roman M. Dubrovin: Russian Academy of Sciences
Atiqa Arshad: Helmholtz-Zentrum Dresden-Rossendorf
Igor Ilyakov: Helmholtz-Zentrum Dresden-Rossendorf
Thales V. A. G. Oliveira: Helmholtz-Zentrum Dresden-Rossendorf
Alexey Ponomaryov: Helmholtz-Zentrum Dresden-Rossendorf
Jan-Christoph Deinert: Helmholtz-Zentrum Dresden-Rossendorf
Sergey Kovalev: Helmholtz-Zentrum Dresden-Rossendorf
Roman V. Pisarev: Russian Academy of Sciences
Mikhail I. Katsnelson: Radboud University
Boris A. Ivanov: Radboud University
Paul H. M. Loosdrecht: University of Cologne
Alexey V. Kimel: Radboud University
Evgeny A. Mashkovich: University of Cologne

Nature Communications, 2024, vol. 15, issue 1, 1-7

Abstract: Abstract Understanding spin-lattice interactions in antiferromagnets is a critical element of the fields of antiferromagnetic spintronics and magnonics. Recently, coherent nonlinear phonon dynamics mediated by a magnon state were discovered in an antiferromagnet. Here, we suggest that a strongly coupled two-magnon-one phonon state in this prototypical system opens a novel pathway to coherently control magnon-phonon dynamics. Utilizing intense narrow-band terahertz (THz) pulses and tunable magnetic fields up to μ0Hext = 7 T, we experimentally realize the conditions of magnon-phonon Fermi resonance in antiferromagnetic CoF2. These conditions imply that both the spin and the lattice anharmonicities harvest energy from the transfer between the subsystems if the magnon eigenfrequency fm is half the frequency of the phonon 2fm = fph. Performing THz pump-infrared probe spectroscopy in conjunction with simulations, we explore the coupled magnon-phonon dynamics in the vicinity of the Fermi-resonance and reveal the corresponding fingerprints of nonlinear interaction facilitating energy exchange between these subsystems.

Date: 2024
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DOI: 10.1038/s41467-024-49716-w

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