Metal-organic framework derived crystalline nanocarbon for Fenton-like reaction

Tingting Lian, Li Xu, Diana Piankova, Jin-Lin Yang, Nadezda V. Tarakina, Yang Wang () and Markus Antonietti
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Tingting Lian: Max Planck Institute of Colloids and Interfaces
Li Xu: University of Science and Technology of China
Diana Piankova: Max Planck Institute of Colloids and Interfaces
Jin-Lin Yang: Nanyang Technological University
Nadezda V. Tarakina: Max Planck Institute of Colloids and Interfaces
Yang Wang: Max Planck Institute of Colloids and Interfaces
Markus Antonietti: Max Planck Institute of Colloids and Interfaces

Nature Communications, 2024, vol. 15, issue 1, 1-10

Abstract: Abstract Nanoporous carbons with tailorable nanoscale texture and long-range ordered structure are promising candidates for energy, environmental and catalytic applications, while the current synthetic methods do not allow elaborate control of local structure. Here we report a salt-assisted strategy to obtain crystalline nanocarbon from direct carbonization of metal-organic frameworks (MOFs). The crystalline product maintains a highly ordered two-dimensional (2D) stacking mode and substantially differs from the traditional weakly ordered patterns of nanoporous carbons upon high-temperature pyrolysis. The MOF-derived crystalline nanocarbon (MCC) comes with a high level of nitrogen and oxygen terminating the 2D layers and shows an impressive performance as a carbocatalyst in Fenton-like reaction for water purification. The successful preparation of MCC illustrates the possibility to discover other crystalline heteroatom-doped carbon phases starting from correctly designed organic precursors and appropriate templating reactions.

Date: 2024
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DOI: 10.1038/s41467-024-50476-w

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