Multiferroicity in plastically deformed SrTiO3

Xi Wang, Anirban Kundu, Bochao Xu, Sajna Hameed, Nadav Rothem, Shai Rabkin, Luka Rogić, Liam Thompson, Alexander McLeod, Martin Greven, Damjan Pelc, Ilya Sochnikov, Beena Kalisky () and Avraham Klein ()
Additional contact information
Xi Wang: Bar-Ilan University
Anirban Kundu: Ariel University
Bochao Xu: University of Connecticut
Sajna Hameed: University of Minnesota
Nadav Rothem: Bar-Ilan University
Shai Rabkin: Bar-Ilan University
Luka Rogić: University of Zagreb
Liam Thompson: University of Minnesota
Alexander McLeod: University of Minnesota
Martin Greven: University of Minnesota
Damjan Pelc: University of Zagreb
Ilya Sochnikov: University of Connecticut
Beena Kalisky: Bar-Ilan University
Avraham Klein: Ariel University

Nature Communications, 2024, vol. 15, issue 1, 1-10

Abstract: Abstract Quantum materials have a fascinating tendency to manifest novel and unexpected electronic states upon proper manipulation. Ideally, such manipulation should induce strong and irreversible changes and lead to new relevant length scales. Plastic deformation introduces large numbers of dislocations into a material, which can organize into extended structures and give rise to qualitatively new physics as a result of the huge localized strains. However, this approach is largely unexplored in the context of quantum materials, which are traditionally grown to be as pristine and clean as possible. Here we show that plastic deformation induces robust magnetism in the quantum paraelectric SrTiO3, a property that is completely absent in the pristine material. We combine scanning magnetic measurements and near-field optical microscopy to find that the magnetic order is localized along dislocation walls and coexists with ferroelectric order along the walls. The magnetic signals can be switched on and off via external stress and altered by external electric fields, which demonstrates that plastically deformed SrTiO3 is a quantum multiferroic. These results establish plastic deformation as a versatile knob for the manipulation of the electronic properties of quantum materials.

Date: 2024
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DOI: 10.1038/s41467-024-51615-z

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