An actuatable ionogel thermoelectric fiber with aligned mesogens-induced thermopower for four-dimensional dynamically adaptive heat harvesting
Liuqi Cao,
Tingting Sun (),
Huiru Zhao,
MengHan Shang,
Lianjun Wang () and
Wan Jiang ()
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Liuqi Cao: Donghua University
Tingting Sun: Donghua University
Huiru Zhao: Donghua University
MengHan Shang: Donghua University
Lianjun Wang: Donghua University
Wan Jiang: Donghua University
Nature Communications, 2025, vol. 16, issue 1, 1-12
Abstract:
Abstract Thermoelectric (TE) ionogel have emerged as promising materials for harvesting low-grade heat owing to their flexibility and giant thermopower. However, current high-performance TE ionogel requires multi-component systems, resulting in trade-offs between TE performance, mechanics, and ion leakage risk. Moreover, the humidity-dependent thermopower and two-dimensional device architectures restrict their practical applications. Here, a thermally actuated TE ionogel fiber is designed by tailoring the interactions between liquid crystal elastomer (LCE) network and ionic liquid. Fine tuning the mesogen orientation of LCE network ensures ~3-fold thermopower boost (25.8 mV K−1) and ~30-fold electrical conductivity boom (21.5 mS m−1) at low humidity (
Date: 2025
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Persistent link: https://EconPapers.repec.org/RePEc:nat:natcom:v:16:y:2025:i:1:d:10.1038_s41467-025-60103-x
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DOI: 10.1038/s41467-025-60103-x
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