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Spectral signature of high-order photon processes enhanced by Cooper-pair pairing

W. C. Smith (), A. Borgognoni, M. Villiers, E. Roverc’h, J. Palomo, M. R. Delbecq, T. Kontos, P. Campagne-Ibarcq, B. Douçot and Z. Leghtas ()
Additional contact information
W. C. Smith: Université PSL, Inria
A. Borgognoni: Université PSL, Inria
M. Villiers: Université PSL, Inria
E. Roverc’h: Université PSL, Inria
J. Palomo: Université PSL, Inria
M. R. Delbecq: Université PSL, Inria
T. Kontos: Université PSL, Inria
P. Campagne-Ibarcq: Université PSL, Inria
B. Douçot: Sorbonne Université and CNRS UMR 7589
Z. Leghtas: Université PSL, Inria

Nature Communications, 2025, vol. 16, issue 1, 1-8

Abstract: Abstract Inducing interactions between individual photons is key for photonic quantum information and studying many-body photon states. Superconducting circuits are well suited to combine strong interactions with low losses. Typically, microwave photons are stored in an LC oscillator shunted by a Josephson junction, where the zero-point phase fluctuations across the junction determine the strength and order of photon interactions. Most superconducting nonlinear oscillators operate with small phase fluctuations, where two-photon Kerr interactions dominate. In our experiment, we shunt a high-impedance LC oscillator with a dipole element favoring the tunneling of paired Cooper pairs. This leads to large phase fluctuations of 3.4, accessing a regime where transition frequencies shift non-monotonically with excitation number. From spectroscopy, we extract two-, three-, and four-photon interaction energies, all of similar strength and exceeding the photon loss rate. Our results open a new regime of high-order photon interactions in microwave quantum optics.

Date: 2025
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DOI: 10.1038/s41467-025-62047-8

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