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Optimization of non-periodic plasmonic light-trapping layers for thin-film solar cells

Ragip A. Pala, John S. Q. Liu, Edward S. Barnard, Daulet Askarov, Erik C. Garnett, Shanhui Fan and Mark L. Brongersma ()
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Ragip A. Pala: Geballe Laboratory for Advanced Materials, Stanford University
John S. Q. Liu: Geballe Laboratory for Advanced Materials, Stanford University
Edward S. Barnard: Geballe Laboratory for Advanced Materials, Stanford University
Daulet Askarov: Geballe Laboratory for Advanced Materials, Stanford University
Erik C. Garnett: Geballe Laboratory for Advanced Materials, Stanford University
Shanhui Fan: Stanford University
Mark L. Brongersma: Geballe Laboratory for Advanced Materials, Stanford University

Nature Communications, 2013, vol. 4, issue 1, 1-7

Abstract: Abstract Non-periodic arrangements of nanoscale light scatterers allow for the realization of extremely effective broadband light-trapping layers for solar cells. However, their optimization is challenging given the massive number of degrees of freedom. Brute-force, full-field electromagnetic simulations are computationally too time intensive to identify high-performance solutions in a vast design space. Here we illustrate how a semi-analytical model can be used to quickly identify promising non-periodic spatial arrangements of nanoscale scatterers. This model only requires basic knowledge of the scattering behaviour of a chosen nanostructure and the waveguiding properties of the semiconductor layer in a cell. Due to its simplicity, it provides new intuition into the ideal amount of disorder in high-performance light-trapping layers. Using simulations and experiments, we demonstrate that arrays of nanometallic stripes featuring a limited amount of disorder, for example, following a quasi-periodic or Fibonacci sequence, can substantially enhance solar absorption over perfectly periodic and random arrays.

Date: 2013
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Persistent link: https://EconPapers.repec.org/RePEc:nat:natcom:v:4:y:2013:i:1:d:10.1038_ncomms3095

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DOI: 10.1038/ncomms3095

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