Restoration of the third law in spin ice thin films
L. Bovo (),
X. Moya,
D. Prabhakaran,
Yeong-Ah Soh,
A.T. Boothroyd,
N.D. Mathur,
G. Aeppli and
S.T. Bramwell
Additional contact information
L. Bovo: University College London, 17-19 Gordon Street
X. Moya: University of Cambridge
D. Prabhakaran: University of Oxford, Clarendon Laboratory, Parks Road
Yeong-Ah Soh: University College London, 17-19 Gordon Street
A.T. Boothroyd: University of Oxford, Clarendon Laboratory, Parks Road
N.D. Mathur: University of Cambridge
G. Aeppli: University College London, 17-19 Gordon Street
S.T. Bramwell: University College London, 17-19 Gordon Street
Nature Communications, 2014, vol. 5, issue 1, 1-8
Abstract:
Abstract A characteristic feature of spin ice is its apparent violation of the third law of thermodynamics. This leads to a number of interesting properties including the emergence of an effective vacuum for magnetic monopoles and their currents – magnetricity. Here we add a new dimension to the experimental study of spin ice by fabricating thin epitaxial films of Dy2Ti2O7, varying between 5 and 60 monolayers on an inert substrate. The films show the distinctive characteristics of spin ice at temperatures >2 K, but at lower temperature we find evidence of a zero entropy state. This restoration of the third law in spin ice thin films is consistent with a predicted strain-induced ordering of a very unusual type, previously discussed for analogous electrical systems. Our results show how the physics of frustrated pyrochlore magnets such as spin ice may be significantly modified in thin-film samples.
Date: 2014
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Persistent link: https://EconPapers.repec.org/RePEc:nat:natcom:v:5:y:2014:i:1:d:10.1038_ncomms4439
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DOI: 10.1038/ncomms4439
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