Coaxial wet-spun yarn supercapacitors for high-energy density and safe wearable electronics
Liang Kou,
Tieqi Huang,
Bingna Zheng,
Yi Han,
Xiaoli Zhao,
Karthikeyan Gopalsamy,
Haiyan Sun and
Chao Gao ()
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Liang Kou: MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Zhejiang University
Tieqi Huang: MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Zhejiang University
Bingna Zheng: MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Zhejiang University
Yi Han: MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Zhejiang University
Xiaoli Zhao: MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Zhejiang University
Karthikeyan Gopalsamy: MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Zhejiang University
Haiyan Sun: MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Zhejiang University
Chao Gao: MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Zhejiang University
Nature Communications, 2014, vol. 5, issue 1, 1-10
Abstract:
Abstract Yarn supercapacitors have great potential in future portable and wearable electronics because of their tiny volume, flexibility and weavability. However, low-energy density limits their development in the area of wearable high-energy density devices. How to enhance their energy densities while retaining their high-power densities is a critical challenge for yarn supercapacitor development. Here we propose a coaxial wet-spinning assembly approach to continuously spin polyelectrolyte-wrapped graphene/carbon nanotube core-sheath fibres, which are used directly as safe electrodes to assembly two-ply yarn supercapacitors. The yarn supercapacitors using liquid and solid electrolytes show ultra-high capacitances of 269 and 177 mF cm−2 and energy densities of 5.91 and 3.84 μWh cm−2, respectively. A cloth supercapacitor superior to commercial capacitor is further interwoven from two individual 40-cm-long coaxial fibres. The combination of scalable coaxial wet-spinning technology and excellent performance of yarn supercapacitors paves the way to wearable and safe electronics.
Date: 2014
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Persistent link: https://EconPapers.repec.org/RePEc:nat:natcom:v:5:y:2014:i:1:d:10.1038_ncomms4754
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DOI: 10.1038/ncomms4754
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