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Coherent properties of single rare-earth spin qubits

P. Siyushev, K. Xia, R. Reuter, M. Jamali, N. Zhao (), N. Yang, C. Duan, N. Kukharchyk, A. D. Wieck, R. Kolesov () and J. Wrachtrup
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P. Siyushev: 3. Physikalisches Institut, Universität Stuttgart and Stuttgart Research Center of Photonic Engineering (SCoPE), Pfaffenwaldring 57
K. Xia: 3. Physikalisches Institut, Universität Stuttgart and Stuttgart Research Center of Photonic Engineering (SCoPE), Pfaffenwaldring 57
R. Reuter: 3. Physikalisches Institut, Universität Stuttgart and Stuttgart Research Center of Photonic Engineering (SCoPE), Pfaffenwaldring 57
M. Jamali: 3. Physikalisches Institut, Universität Stuttgart and Stuttgart Research Center of Photonic Engineering (SCoPE), Pfaffenwaldring 57
N. Zhao: Beijing Computational Science Research Center
N. Yang: Institute of Applied Physics and Computational Mathematics
C. Duan: Hefei National Laboratory for Physics Sciences at Microscale, University of Science and Technology of China
N. Kukharchyk: Ruhr-Universität Bochum
A. D. Wieck: Ruhr-Universität Bochum
R. Kolesov: 3. Physikalisches Institut, Universität Stuttgart and Stuttgart Research Center of Photonic Engineering (SCoPE), Pfaffenwaldring 57
J. Wrachtrup: 3. Physikalisches Institut, Universität Stuttgart and Stuttgart Research Center of Photonic Engineering (SCoPE), Pfaffenwaldring 57

Nature Communications, 2014, vol. 5, issue 1, 1-6

Abstract: Abstract Rare-earth-doped crystals are excellent hardware for quantum storage of photons. Additional functionality of these materials is added by their waveguiding properties allowing for on-chip photonic networks. However, detection and coherent properties of rare-earth single-spin qubits have not been demonstrated so far. Here we present experimental results on high-fidelity optical initialization, effcient coherent manipulation and optical readout of a single-electron spin of Ce3+ ion in a yttrium aluminium garnet crystal. Under dynamic decoupling, spin coherence lifetime reaches T2=2 ms and is almost limited by the measured spin-lattice relaxation time T1=4.5 ms. Strong hyperfine coupling to aluminium nuclear spins suggests that cerium electron spins can be exploited as an interface between photons and long-lived nuclear spin memory. Combined with high brightness of Ce3+ emission and a possibility of creating photonic circuits out of the host material, this makes cerium spins an interesting option for integrated quantum photonics.

Date: 2014
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DOI: 10.1038/ncomms4895

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