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Ultrafast optical tuning of ferromagnetism via the carrier density

Masakazu Matsubara (), Alexander Schroer, Andreas Schmehl, Alexander Melville, Carsten Becher, Mauricio Trujillo-Martinez, Darrell G. Schlom, Jochen Mannhart, Johann Kroha and Manfred Fiebig
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Masakazu Matsubara: Tohoku University
Alexander Schroer: Physikalisches Institut, Universität Bonn
Andreas Schmehl: Institut für Physik, Universität Augsburg
Alexander Melville: Cornell University
Carsten Becher: ETH Zurich
Mauricio Trujillo-Martinez: Physikalisches Institut, Universität Bonn
Darrell G. Schlom: Cornell University
Jochen Mannhart: Max Planck Institute for Solid State Research
Johann Kroha: Physikalisches Institut, Universität Bonn
Manfred Fiebig: ETH Zurich

Nature Communications, 2015, vol. 6, issue 1, 1-7

Abstract: Abstract Interest in manipulating the magnetic order by ultrashort laser pulses has thrived since it was observed that such pulses can be used to alter the magnetization on a sub-picosecond timescale. Usually this involves demagnetization by laser heating or, in rare cases, a transient increase of magnetization. Here we demonstrate a mechanism that allows the magnetic order of a material to be enhanced or attenuated at will. This is possible in systems simultaneously possessing a low, tunable density of conduction band carriers and a high density of magnetic moments. In such systems, the thermalization time can be set such that adiabatic processes dominate the photoinduced change of the magnetic order—the three-temperature model for interacting thermalized electron, spin and lattice reservoirs is bypassed. In ferromagnetic Eu1−xGdxO, we thereby demonstrate the strengthening as well as the weakening of the magnetic order by ~10% and within ≤3 ps by optically controlling the magnetic exchange interaction.

Date: 2015
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Persistent link: https://EconPapers.repec.org/RePEc:nat:natcom:v:6:y:2015:i:1:d:10.1038_ncomms7724

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DOI: 10.1038/ncomms7724

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