Atomically resolved real-space imaging of hot electron dynamics
D. Lock,
K. R. Rusimova,
T. L. Pan,
R. E. Palmer and
P. A. Sloan ()
Additional contact information
D. Lock: University of Bath
K. R. Rusimova: University of Bath
T. L. Pan: Nanoscale Physics Research Laboratory, School of Physics and Astronomy, University of Birmingham
R. E. Palmer: Nanoscale Physics Research Laboratory, School of Physics and Astronomy, University of Birmingham
P. A. Sloan: University of Bath
Nature Communications, 2015, vol. 6, issue 1, 1-7
Abstract:
Abstract The dynamics of hot electrons are central to understanding the properties of many electronic devices. But their ultra-short lifetime, typically 100 fs or less, and correspondingly short transport length-scale in the nanometre range constrain real-space investigations. Here we report variable temperature and voltage measurements of the nonlocal manipulation of adsorbed molecules on the Si(111)-7 × 7 surface in the scanning tunnelling microscope. The range of the nonlocal effect increases with temperature and, at constant temperature, is invariant over a wide range of electron energies. The measurements probe, in real space, the underlying hot electron dynamics on the 10 nm scale and are well described by a two-dimensional diffusive model with a single decay channel, consistent with 2-photon photo-emission (2PPE) measurements of the real time dynamics.
Date: 2015
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Persistent link: https://EconPapers.repec.org/RePEc:nat:natcom:v:6:y:2015:i:1:d:10.1038_ncomms9365
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DOI: 10.1038/ncomms9365
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