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Quantum electric-dipole liquid on a triangular lattice

Shi-Peng Shen, Jia-Chuan Wu, Jun-Da Song, Xue-Feng Sun (), Yi-Feng Yang, Yi-Sheng Chai, Da-Shan Shang, Shou-Guo Wang, James F. Scott and Young Sun ()
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Shi-Peng Shen: Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences
Jia-Chuan Wu: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China
Jun-Da Song: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China
Xue-Feng Sun: Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China
Yi-Feng Yang: Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences
Yi-Sheng Chai: Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences
Da-Shan Shang: Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences
Shou-Guo Wang: Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences
James F. Scott: Cavendish Laboratory, University of Cambridge
Young Sun: Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences

Nature Communications, 2016, vol. 7, issue 1, 1-6

Abstract: Abstract Geometric frustration and quantum fluctuations may prohibit the formation of long-range ordering even at the lowest temperature, and therefore liquid-like ground states could be expected. A good example is the quantum spin liquid in frustrated magnets. Geometric frustration and quantum fluctuations can happen beyond magnetic systems. Here we propose that quantum electric-dipole liquids, analogues of quantum spin liquids, could emerge in frustrated dielectrics where antiferroelectrically coupled electric dipoles reside on a triangular lattice. The quantum paraelectric hexaferrite BaFe12O19 with geometric frustration represents a promising candidate for the proposed electric-dipole liquid. We present a series of experimental lines of evidence, including dielectric permittivity, heat capacity and thermal conductivity measured down to 66 mK, to reveal the existence of an unusual liquid-like quantum phase in BaFe12O19, characterized by itinerant low-energy excitations with a small gap. The possible quantum liquids of electric dipoles in frustrated dielectrics open up a fresh playground for fundamental physics.

Date: 2016
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DOI: 10.1038/ncomms10569

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