Tailoring the chiral magnetic interaction between two individual atoms

A. A. Khajetoorians (), M. Steinbrecher, M. Ternes, M. Bouhassoune, M. dos Santos Dias, S. Lounis, J. Wiebe () and R. Wiesendanger
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A. A. Khajetoorians: Hamburg University
M. Steinbrecher: Hamburg University
M. Ternes: Max Planck Institute for Solid State Research
M. Bouhassoune: Peter Grünberg Institut and Institute for Advanced Simulation, Forschungszentrum Jülich & JARA
M. dos Santos Dias: Peter Grünberg Institut and Institute for Advanced Simulation, Forschungszentrum Jülich & JARA
S. Lounis: Peter Grünberg Institut and Institute for Advanced Simulation, Forschungszentrum Jülich & JARA
J. Wiebe: Hamburg University
R. Wiesendanger: Hamburg University

Nature Communications, 2016, vol. 7, issue 1, 1-8

Abstract: Abstract Chiral magnets are a promising route towards dense magnetic storage technology due to their inherent nano-scale dimensions and energy efficient properties. Engineering chiral magnets requires atomic-level control of the magnetic exchange interactions, including the Dzyaloshinskii–Moriya interaction, which defines a rotational sense for the magnetization of two coupled magnetic moments. Here we show that the indirect conduction electron-mediated Dzyaloshinskii–Moriya interaction between two individual magnetic atoms on a metallic surface can be manipulated by changing the interatomic distance with the tip of a scanning tunnelling microscope. We quantify this interaction by comparing our measurements to a quantum magnetic model and ab-initio calculations yielding a map of the chiral ground states of pairs of atoms depending on the interatomic separation. The map enables tailoring the chirality of the magnetization in dilute atomic-scale magnets.

Date: 2016
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DOI: 10.1038/ncomms10620

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