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High-harmonic generation by field enhanced femtosecond pulses in metal-sapphire nanostructure

Seunghwoi Han, Hyunwoong Kim, Yong Woo Kim, Young-Jin Kim, Seungchul Kim, In-Yong Park and Seung-Woo Kim ()
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Seunghwoi Han: Korea Advanced Institute of Science and Technology (KAIST)
Hyunwoong Kim: Korea Advanced Institute of Science and Technology (KAIST)
Yong Woo Kim: Korea Advanced Institute of Science and Technology (KAIST)
Young-Jin Kim: School of Mechanical and Aerospace Engineering, Nanyang Technological University (NTU)
Seungchul Kim: Max Planck Center for Attosecond Science, Max Planck POSTECH/KOREA Res. Initiative
In-Yong Park: Korea Research Institute of Standards and Science (KRISS)
Seung-Woo Kim: Korea Advanced Institute of Science and Technology (KAIST)

Nature Communications, 2016, vol. 7, issue 1, 1-7

Abstract: Abstract Plasmonic high-harmonic generation (HHG) drew attention as a means of producing coherent extreme ultraviolet (EUV) radiation by taking advantage of field enhancement occurring in metallic nanostructures. Here a metal-sapphire nanostructure is devised to provide a solid tip as the HHG emitter, replacing commonly used gaseous atoms. The fabricated solid tip is made of monocrystalline sapphire surrounded by a gold thin-film layer, and intended to produce EUV harmonics by the inter- and intra-band oscillations of electrons driven by the incident laser. The metal-sapphire nanostructure enhances the incident laser field by means of surface plasmon polaritons, triggering HHG directly from moderate femtosecond pulses of ∼0.1 TW cm−2 intensities. The measured EUV spectra exhibit odd-order harmonics up to ∼60 nm wavelengths without the plasma atomic lines typically seen when using gaseous atoms as the HHG emitter. This experimental outcome confirms that the plasmonic HHG approach is a promising way to realize coherent EUV sources for nano-scale near-field applications in spectroscopy, microscopy, lithography and atto-second physics.

Date: 2016
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Persistent link: https://EconPapers.repec.org/RePEc:nat:natcom:v:7:y:2016:i:1:d:10.1038_ncomms13105

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DOI: 10.1038/ncomms13105

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