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Field induced spontaneous quasiparticle decay and renormalization of quasiparticle dispersion in a quantum antiferromagnet

Tao Hong (), Y. Qiu, M. Matsumoto, D. A. Tennant, K. Coester, K. P. Schmidt, F. F. Awwadi, M. M. Turnbull, H. Agrawal and A. L. Chernyshev
Additional contact information
Tao Hong: Oak Ridge National Laboratory
Y. Qiu: National Institute of Standards and Technology
M. Matsumoto: Shizuoka University
D. A. Tennant: Oak Ridge National Laboratory
K. Coester: Lehrstuhl für Theoretische Physik I, TU Dortmund
K. P. Schmidt: Lehrstuhl für Theoretische Physik I
F. F. Awwadi: The University of Jordan
M. M. Turnbull: Carlson School of Chemistry and Biochemistry, Clark University
H. Agrawal: Oak Ridge National Laboratory
A. L. Chernyshev: University of California

Nature Communications, 2017, vol. 8, issue 1, 1-8

Abstract: Abstract The notion of a quasiparticle, such as a phonon, a roton or a magnon, is used in modern condensed matter physics to describe an elementary collective excitation. The intrinsic zero-temperature magnon damping in quantum spin systems can be driven by the interaction of the one-magnon states and multi-magnon continuum. However, detailed experimental studies on this quantum many-body effect induced by an applied magnetic field are rare. Here we present a high-resolution neutron scattering study in high fields on an S=1/2 antiferromagnet C9H18N2CuBr4. Compared with the non-interacting linear spin–wave theory, our results demonstrate a variety of phenomena including field-induced renormalization of one-magnon dispersion, spontaneous magnon decay observed via intrinsic linewidth broadening, unusual non-Lorentzian two-peak structure in the excitation spectra and a dramatic shift of spectral weight from one-magnon state to the two-magnon continuum.

Date: 2017
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DOI: 10.1038/ncomms15148

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