All-optical control and super-resolution imaging of quantum emitters in layered materials
Mehran Kianinia,
Carlo Bradac (),
Bernd Sontheimer,
Fan Wang,
Toan Trong Tran,
Minh Nguyen,
Sejeong Kim,
Zai-Quan Xu,
Dayong Jin,
Andreas W. Schell,
Charlene J. Lobo,
Igor Aharonovich () and
Milos Toth ()
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Mehran Kianinia: University of Technology Sydney
Carlo Bradac: University of Technology Sydney
Bernd Sontheimer: Humboldt-Universität zu Berlin
Fan Wang: University of Technology Sydney
Toan Trong Tran: University of Technology Sydney
Minh Nguyen: University of Technology Sydney
Sejeong Kim: University of Technology Sydney
Zai-Quan Xu: University of Technology Sydney
Dayong Jin: University of Technology Sydney
Andreas W. Schell: Kyoto University
Charlene J. Lobo: University of Technology Sydney
Igor Aharonovich: University of Technology Sydney
Milos Toth: University of Technology Sydney
Nature Communications, 2018, vol. 9, issue 1, 1-8
Abstract:
Abstract Layered van der Waals materials are emerging as compelling two-dimensional platforms for nanophotonics, polaritonics, valleytronics and spintronics, and have the potential to transform applications in sensing, imaging and quantum information processing. Among these, hexagonal boron nitride (hBN) is known to host ultra-bright, room-temperature quantum emitters, whose nature is yet to be fully understood. Here we present a set of measurements that give unique insight into the photophysical properties and level structure of hBN quantum emitters. Specifically, we report the existence of a class of hBN quantum emitters with a fast-decaying intermediate and a long-lived metastable state accessible from the first excited electronic state. Furthermore, by means of a two-laser repumping scheme, we show an enhanced photoluminescence and emission intensity, which can be utilized to realize a new modality of far-field super-resolution imaging. Our findings expand current understanding of quantum emitters in hBN and show new potential ways of harnessing their nonlinear optical properties in sub-diffraction nanoscopy.
Date: 2018
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Persistent link: https://EconPapers.repec.org/RePEc:nat:natcom:v:9:y:2018:i:1:d:10.1038_s41467-018-03290-0
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DOI: 10.1038/s41467-018-03290-0
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