Ultra-narrow-band near-infrared thermal exciton radiation in intrinsic one-dimensional semiconductors

Taishi Nishihara, Akira Takakura, Yuhei Miyauchi () and Kenichiro Itami ()
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Taishi Nishihara: Nagoya University
Akira Takakura: Nagoya University
Yuhei Miyauchi: Nagoya University
Kenichiro Itami: Nagoya University

Nature Communications, 2018, vol. 9, issue 1, 1-7

Abstract: Abstract Thermal radiation is the most primitive light emission phenomenon of materials. Broadband radiation from red-hot materials is well known as the kick-starter phenomenon of modern quantum physics in the early twentieth century; even nowadays, its artificial control plays a central role in modern science and technology. Herein, we report the fundamental thermal radiation properties of intrinsic one-dimensional semiconductors and metals, which have not been elucidated because of significant technical challenges. We observed narrow-band near-infrared radiation from semiconducting single-walled carbon nanotubes at 1000–2000 K in contrast to its broadband metallic counterpart. We confirm that the ultra-narrow-band radiation is enabled by the thermal generation of excitons that are hydrogen-like neutral exotic atoms comprising mutually bound electrons and holes. Our findings uncover the robust quantum correlations in intrinsic one-dimensional semiconductors even at 2000 K; additionally, the findings provide an opportunity for excitonic optothermal engineering toward the realization of efficient thermophotovoltaic energy harvesting.

Date: 2018
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DOI: 10.1038/s41467-018-05598-3

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