Stable cycling of high-voltage lithium metal batteries in ether electrolytes

Shuhong Jiao, Xiaodi Ren, Ruiguo Cao, Mark H. Engelhard, Yuzi Liu, Dehong Hu, Donghai Mei, Jianming Zheng, Wengao Zhao, Qiuyan Li, Ning Liu, Brian D. Adams, Cheng Ma, Jun Liu, Ji-Guang Zhang () and Wu Xu ()
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Shuhong Jiao: Energy and Environment Directorate, Pacific Northwest National Laboratory
Xiaodi Ren: Energy and Environment Directorate, Pacific Northwest National Laboratory
Ruiguo Cao: Energy and Environment Directorate, Pacific Northwest National Laboratory
Mark H. Engelhard: Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory
Yuzi Liu: Centre for Nanoscale Materials, Argonne National Laboratory
Dehong Hu: Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory
Donghai Mei: Physical and Computational Directorate, Pacific Northwest National Laboratory
Jianming Zheng: Energy and Environment Directorate, Pacific Northwest National Laboratory
Wengao Zhao: Energy and Environment Directorate, Pacific Northwest National Laboratory
Qiuyan Li: Energy and Environment Directorate, Pacific Northwest National Laboratory
Ning Liu: Physical and Computational Directorate, Pacific Northwest National Laboratory
Brian D. Adams: Energy and Environment Directorate, Pacific Northwest National Laboratory
Cheng Ma: University of Science and Technology of China
Jun Liu: Energy and Environment Directorate, Pacific Northwest National Laboratory
Ji-Guang Zhang: Energy and Environment Directorate, Pacific Northwest National Laboratory
Wu Xu: Energy and Environment Directorate, Pacific Northwest National Laboratory

Nature Energy, 2018, vol. 3, issue 9, 739-746

Abstract: Abstract The key to enabling long-term cycling stability of high-voltage lithium (Li) metal batteries is the development of functional electrolytes that are stable against both Li anodes and high-voltage (above 4 V versus Li/Li+) cathodes. Due to their limited oxidative stability ( 90% over 300 cycles and ~80% over 500 cycles with a charge cut-off voltage of 4.3 V. This study offers a promising approach to enable ether-based electrolytes for high-voltage Li metal battery applications.

Date: 2018
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DOI: 10.1038/s41560-018-0199-8

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