Scalable two-terminal all-perovskite tandem solar modules with a 19.1% efficiency
Bahram Abdollahi Nejand (),
David B. Ritzer,
Hang Hu,
Fabian Schackmar,
Somayeh Moghadamzadeh,
Thomas Feeney,
Roja Singh,
Felix Laufer,
Raphael Schmager,
Raheleh Azmi,
Milian Kaiser,
Tobias Abzieher,
Saba Gharibzadeh,
Erik Ahlswede,
Uli Lemmer,
Bryce S. Richards and
Ulrich W. Paetzold ()
Additional contact information
Bahram Abdollahi Nejand: Karlsruhe Institute of Technology
David B. Ritzer: Karlsruhe Institute of Technology
Hang Hu: Karlsruhe Institute of Technology
Fabian Schackmar: Karlsruhe Institute of Technology
Somayeh Moghadamzadeh: Karlsruhe Institute of Technology
Thomas Feeney: Karlsruhe Institute of Technology
Roja Singh: Karlsruhe Institute of Technology
Felix Laufer: Karlsruhe Institute of Technology
Raphael Schmager: Karlsruhe Institute of Technology
Raheleh Azmi: Karlsruhe Institute of Technology (KIT)
Milian Kaiser: Karlsruhe Institute of Technology
Tobias Abzieher: Karlsruhe Institute of Technology
Saba Gharibzadeh: Karlsruhe Institute of Technology
Erik Ahlswede: Center for Solar Energy and Hydrogen Research Baden-Württemberg (ZSW)
Uli Lemmer: Karlsruhe Institute of Technology
Bryce S. Richards: Karlsruhe Institute of Technology
Ulrich W. Paetzold: Karlsruhe Institute of Technology
Nature Energy, 2022, vol. 7, issue 7, 620-630
Abstract:
Abstract Monolithic all-perovskite tandem photovoltaics promise to combine low-cost and high-efficiency solar energy harvesting with the advantages of all-thin-film technologies. To date, laboratory-scale all-perovskite tandem solar cells have only been fabricated using non-scalable fabrication techniques. In response, this work reports on laser-scribed all-perovskite tandem modules processed exclusively with scalable fabrication methods (blade coating and vacuum deposition), demonstrating power conversion efficiencies up to 19.1% (aperture area, 12.25 cm2; geometric fill factor, 94.7%) and stable power output. Compared to the performance of our spin-coated reference tandem solar cells (efficiency, 23.5%; area, 0.1 cm2), our prototypes demonstrate substantial advances in the technological readiness of all-perovskite tandem photovoltaics. By means of electroluminescence imaging and laser-beam-induced current mapping, we demonstrate the homogeneous current collection in both subcells over the entire module area, which explains low losses (
Date: 2022
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DOI: 10.1038/s41560-022-01059-w
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