Preserving order by controlled disorder

Timo Boehler and Dominic Bresser ()
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Timo Boehler: Helmholtz Institute Ulm (HIU)
Dominic Bresser: Helmholtz Institute Ulm (HIU)

Nature Energy, 2024, vol. 9, issue 10, 1181-1182

Abstract: Nickel-rich lithium-ion cathode materials face severe structural and interfacial instabilities when cycled at high potentials and high degrees of delithiation. Now, a LiNi0.8Mn0.1Co0.1O2 material with a complementary composition and structure gradient, composed of an ordered, layered Co-poor bulk phase and a Co-enriched disordered rock-salt surface layer, is shown to efficiently address the issues.

Date: 2024
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DOI: 10.1038/s41560-024-01628-1

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