Benchmarking the reproducibility of all-solid-state battery cell performance

Sebastian Puls, Elina Nazmutdinova, Fariza Kalyk, Henry M. Woolley, Jesper Frost Thomsen, Zhu Cheng, Adrien Fauchier-Magnan, Ajay Gautam, Michael Gockeln, So-Yeon Ham, Md Toukir Hasan, Min-Gi Jeong, Daiki Hiraoka, Jong Seok Kim, Tobias Kutsch, Barthélémy Lelotte, Philip Minnmann, Vanessa Miß, Kota Motohashi, Douglas Lars Nelson, Frans Ooms, Francesco Piccolo, Christian Plank, Maria Rosner, Stephanie E. Sandoval, Eva Schlautmann, Robin Schuster, Dominic Spencer-Jolly, Yipeng Sun, Bairav S. Vishnugopi, Ruizhuo Zhang, Huang Zheng, Philipp Adelhelm, Torsten Brezesinski, Peter G. Bruce, Michael Danzer, Mario El Kazzi, Hubert Gasteiger, Kelsey B. Hatzell, Akitoshi Hayashi, Felix Hippauf, Jürgen Janek, Yoon Seok Jung, Matthew T. McDowell, Ying Shirley Meng, Partha P. Mukherjee, Saneyuki Ohno, Bernhard Roling, Atsushi Sakuda, Julian Schwenzel, Xueliang Sun, Claire Villevieille, Marnix Wagemaker, Wolfgang G. Zeier and Nella M. Vargas-Barbosa ()
Additional contact information
Sebastian Puls: Forschungszetrum Jülich
Elina Nazmutdinova: University of Münster
Fariza Kalyk: Forschungszetrum Jülich
Henry M. Woolley: University of Münster
Jesper Frost Thomsen: University of Münster
Zhu Cheng: Delft University of Technology
Adrien Fauchier-Magnan: LEPMI
Ajay Gautam: Delft University of Technology
Michael Gockeln: Fraunhofer Institute for Manufacturing and Advanced Materials IFAM
So-Yeon Ham: University of California San Diego
Md Toukir Hasan: Purdue University
Min-Gi Jeong: Department of Mechanical and Aerospace Engineering and the Andlinger Center for Energy and the Environment
Daiki Hiraoka: Osaka Metropolitan University
Jong Seok Kim: Yonsei University
Tobias Kutsch: Technische Universität München
Barthélémy Lelotte: Paul Scherrer Institut
Philip Minnmann: Justus Liebig University Giessen
Vanessa Miß: Philipps-Universität Marburg
Kota Motohashi: Osaka Metropolitan University
Douglas Lars Nelson: Georgia Institute of Technology
Frans Ooms: Delft University of Technology
Francesco Piccolo: Humboldt Universität zu Berlin
Christian Plank: University of Bayreuth
Maria Rosner: Fraunhofer Institute for Material and Beam Technology (IWS)
Stephanie E. Sandoval: Georgia Institute of Technology
Eva Schlautmann: University of Münster
Robin Schuster: Technische Universität München
Dominic Spencer-Jolly: University of Oxford
Yipeng Sun: University of Western Ontario
Bairav S. Vishnugopi: Purdue University
Ruizhuo Zhang: Karlsruhe Institute of Technology (KIT)
Huang Zheng: Kyushu University
Philipp Adelhelm: Humboldt Universität zu Berlin
Torsten Brezesinski: Karlsruhe Institute of Technology (KIT)
Peter G. Bruce: University of Oxford
Michael Danzer: University of Bayreuth
Mario El Kazzi: Paul Scherrer Institut
Hubert Gasteiger: Technische Universität München
Kelsey B. Hatzell: Department of Mechanical and Aerospace Engineering and the Andlinger Center for Energy and the Environment
Akitoshi Hayashi: Osaka Metropolitan University
Felix Hippauf: Fraunhofer Institute for Material and Beam Technology (IWS)
Jürgen Janek: Justus Liebig University Giessen
Yoon Seok Jung: Yonsei University
Matthew T. McDowell: Georgia Institute of Technology
Ying Shirley Meng: University of California San Diego
Partha P. Mukherjee: Purdue University
Saneyuki Ohno: Kyushu University
Bernhard Roling: Philipps-Universität Marburg
Atsushi Sakuda: Osaka Metropolitan University
Julian Schwenzel: Fraunhofer Institute for Manufacturing and Advanced Materials IFAM
Xueliang Sun: University of Western Ontario
Claire Villevieille: LEPMI
Marnix Wagemaker: Delft University of Technology
Wolfgang G. Zeier: Forschungszetrum Jülich
Nella M. Vargas-Barbosa: Forschungszetrum Jülich

Nature Energy, 2024, vol. 9, issue 10, 1310-1320

Abstract: Abstract The interlaboratory comparability and reproducibility of all-solid-state battery cell cycling performance are poorly understood due to the lack of standardized set-ups and assembly parameters. This study quantifies the extent of this variability by providing commercially sourced battery materials—LiNi0.6Mn0.2Co0.2O2 for the positive electrode, Li6PS5Cl as the solid electrolyte and indium for the negative electrode—to 21 research groups. Each group was asked to use their own cell assembly protocol but follow a specific electrochemical protocol. The results show large variability in assembly and electrochemical performance, including differences in processing pressures, pressing durations and In-to-Li ratios. Despite this, an initial open circuit voltage of 2.5 and 2.7 V vs Li+/Li is a good predictor of successful cycling for cells using these electroactive materials. We suggest a set of parameters for reporting all-solid-state battery cycling results and advocate for reporting data in triplicate.

Date: 2024
References: View references in EconPapers View complete reference list from CitEc
Citations: View citations in EconPapers (1)

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DOI: 10.1038/s41560-024-01634-3

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