Symmetry-dependent Mn-magnetism in Al 69.8 Pd 12.1 Mn 18.1
D. Rau,
J. L. Gavilano (),
C. Beeli,
J. Hinderer,
E. Felder,
G. A. Wigger and
H. R. Ott
The European Physical Journal B: Condensed Matter and Complex Systems, 2005, vol. 46, issue 2, 281-287
Abstract:
We investigated the stability of magnetic moments in Al 69.8 Pd 12.1 Mn 18. 1 . This alloy exists in both, the icosahedral (i) and the decagonal (d) quasicrystalline form. The transition from the i- to the d-phase is achieved by a simple heat treatment. We present the results of measurements of the 27 Al NMR-response, the dc magnetic susceptibility, and the low-temperature specific heat of both phases. In the icosahedral compound, the majority of the Mn ions carries a magnetic moment. Their number is reduced by approximately a factor of two by transforming the alloy to its decagonal variety. For both compounds, we have indications for two different local environments of the Al nuclei. The first reflects a low density of states of conduction electrons and a weak coupling of the Al nuclei to the Mn-moments. The second type of environment implies a large d-electron density of states at the Fermi level and a strong coupling to the magnetic Mn moments. Spin-glass freezing transitions are observed at T deca f =12 K for the decagonal, and T ico f =19 K for the icosahedral phase. Copyright EDP Sciences/Società Italiana di Fisica/Springer-Verlag 2005
Date: 2005
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Persistent link: https://EconPapers.repec.org/RePEc:spr:eurphb:v:46:y:2005:i:2:p:281-287
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DOI: 10.1140/epjb/e2005-00245-9
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