VALENCE- AND INNER-SHELL SPECTROSCOPY ON RARE-GAS CLUSTERS

O. Björneholm, F. Federmann, M. Joppien, F. Fössing, S. Kakar, R. von Pietrowski and T. Möller
Additional contact information
O. Björneholm: Hamburger Synchrotronstrahlungslabor HASYLAB at Deutsches Elektronensynchrotron DESY, 22607 Hamburg, Notkestr. 85, Germany
F. Federmann: Hamburger Synchrotronstrahlungslabor HASYLAB at Deutsches Elektronensynchrotron DESY, 22607 Hamburg, Notkestr. 85, Germany
M. Joppien: Hamburger Synchrotronstrahlungslabor HASYLAB at Deutsches Elektronensynchrotron DESY, 22607 Hamburg, Notkestr. 85, Germany;
F. Fössing: Hamburger Synchrotronstrahlungslabor HASYLAB at Deutsches Elektronensynchrotron DESY, 22607 Hamburg, Notkestr. 85, Germany;
S. Kakar: Hamburger Synchrotronstrahlungslabor HASYLAB at Deutsches Elektronensynchrotron DESY, 22607 Hamburg, Notkestr. 85, Germany
R. von Pietrowski: Hamburger Synchrotronstrahlungslabor HASYLAB at Deutsches Elektronensynchrotron DESY, 22607 Hamburg, Notkestr. 85, Germany;
T. Möller: Hamburger Synchrotronstrahlungslabor HASYLAB at Deutsches Elektronensynchrotron DESY, 22607 Hamburg, Notkestr. 85, Germany

Surface Review and Letters (SRL), 1996, vol. 03, issue 01, 299-306

Abstract: An overview of the present status of valence- and inner-shell spectroscopy on rare-gas clusters is given. Fluorescence excitation, time-of-flight ion and photoelectron spectroscopy with synchrotron excitation was used to study the electronic level structure of rare-gas clusters. Ne and Ar clusters covering the size range from the monomer up to a few thousand atoms/cluster are used as examples. Specific advantages and limitations of different methods of the study of electronic level structure as well as geometrical structure are discussed. A wealth of information on the evolution of electronic level structure has already been obtained. Nevertheless, several interesting questions concerning the evolution of energy-level shifts remain unresolved. Prospects for future work and experimental developments are given.

Date: 1996
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DOI: 10.1142/S0218625X96000553

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