PROTON TUNNELING IN THE S1STATE OF TROPOLONE–M1(M=Ar,Kr,Xe,CH4,CD4,N2)CLUSTERS

H. Sekiya, H. Hamabe, T. Nakajima and Y. Nishimura
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H. Sekiya: Institute of Advanced Material Study, and Department of Molecular Science and Technology, Graduate School of Engineering Sciences, Kyushu University, Kasuga-shi, Fukuoka 816, Japan
H. Hamabe: Institute of Advanced Material Study, and Department of Molecular Science and Technology, Graduate School of Engineering Sciences, Kyushu University, Kasuga-shi, Fukuoka 816, Japan
T. Nakajima: Institute of Advanced Material Study, and Department of Molecular Science and Technology, Graduate School of Engineering Sciences, Kyushu University, Kasuga-shi, Fukuoka 816, Japan
Y. Nishimura: Institute of Advanced Material Study, and Department of Molecular Science and Technology, Graduate School of Engineering Sciences, Kyushu University, Kasuga-shi, Fukuoka 816, Japan

Surface Review and Letters (SRL), 1996, vol. 03, issue 01, 493-497

Abstract: TheS1←S0fluorescence excitation spectra of jet-cooled tropolone–M1(M=Ar,Kr,Xe,CH4,CD4,N2)clusters have been measured to investigate the effect of intermolecular interactions on proton tunneling. It has been found that the${\rm O}_0^0 $tunneling splittings of tropolone–CH4/CD4and tropolone–N2are significantly smaller than that of tropolone.

Date: 1996
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DOI: 10.1142/S0218625X96000899

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