DRAMATIC EFFECT ON LITHIUM-CLUSTER EVAPORATION: THE EXAMPLE OF${\rm Li}_{11}^+$

R. Antoine, D. Rayane, Ph. Dugourd, B. Vezin, B. Tribollet and M. Broyer
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R. Antoine: Laboratoire de Spectromérie Ionique et Moléculaire (URA CNRS n° 171), Université Lyon 1, Bât. 205, 43 Bd du 11 Novembre, 1918 - 69622 Villeurbanne Cedex, France
D. Rayane: Laboratoire de Spectromérie Ionique et Moléculaire (URA CNRS n° 171), Université Lyon 1, Bât. 205, 43 Bd du 11 Novembre, 1918 - 69622 Villeurbanne Cedex, France
Ph. Dugourd: Laboratoire de Spectromérie Ionique et Moléculaire (URA CNRS n° 171), Université Lyon 1, Bât. 205, 43 Bd du 11 Novembre, 1918 - 69622 Villeurbanne Cedex, France
B. Vezin: Laboratoire de Spectromérie Ionique et Moléculaire (URA CNRS n° 171), Université Lyon 1, Bât. 205, 43 Bd du 11 Novembre, 1918 - 69622 Villeurbanne Cedex, France
B. Tribollet: Laboratoire de Spectromérie Ionique et Moléculaire (URA CNRS n° 171), Université Lyon 1, Bât. 205, 43 Bd du 11 Novembre, 1918 - 69622 Villeurbanne Cedex, France
M. Broyer: Laboratoire de Spectromérie Ionique et Moléculaire (URA CNRS n° 171), Université Lyon 1, Bât. 205, 43 Bd du 11 Novembre, 1918 - 69622 Villeurbanne Cedex, France

Surface Review and Letters (SRL), 1996, vol. 03, issue 01, 545-549

Abstract: We have studied the unimolecular evaporation of ionized lithium clusters for different conditions of ionization. In this article we present the total evaporative rates and the monomer–dimer branching ratios for${\rm Li}_{11}^+$. We observe nonstatistical effects, associated with the dissociation along a less energetically favorable channel. Even after a few microseconds, the internal energy is probably not statistically distributed in all the vibrational modes.

Date: 1996
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DOI: 10.1142/S0218625X96000991

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