SPECTROSCOPY AND EXCITED-STATE DYNAMICS OF BENZENE-TRIMER ION

K. Ohashi, Y. Nakai, T. Shibata and N. Nishi
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K. Ohashi: Department of Chemistry, Faculty of Science, Kyushu University, Hakozaki, Fukuoka 812, Japan
Y. Nakai: Department of Chemistry, Faculty of Science, Kyushu University, Hakozaki, Fukuoka 812, Japan
T. Shibata: Department of Chemistry, Faculty of Science, Kyushu University, Hakozaki, Fukuoka 812, Japan
N. Nishi: Department of Chemistry, Faculty of Science, Kyushu University, Hakozaki, Fukuoka 812, Japan

Surface Review and Letters (SRL), 1996, vol. 03, issue 01, 601-605

Abstract: The photodissociation of(C6H6)3+is studied in the rangehν=0.9–3.0eV. The electronic spectrum of(C6H6)3+shows the main band athν≈1.29eVand a side band at ≈1.02 eV. The(C6H6)3+ion retains spectroscopic features characteristic of(C6H6)2+, suggesting that the positive charge is carried by a dimer subunit in(C6H6)3+. The major fragment ion changes smoothly from(C6H6)2+toC6H6+with increasing photon energy from 0.9 to 1.8 eV. The product branching ratios and the kinetic energy of theC6H6+fragment are consistent with a two-step model for the formation ofC6H6+.

Date: 1996
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DOI: 10.1142/S0218625X9600108X

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