SINGLE-PHOTON IONIZATION OF THE PRIMARY PHOTOFRAGMENTS OF CHLORINE MONOXIDE

R. Flesch, J. Plenge, M.-C. Schürmann, S. Kühl, M. Klusmann and E. Rühl
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R. Flesch: Fachbereich Physik, Universität Osnabrück, Barbarastr. 7, 49069 Osnabrück, Germany
J. Plenge: Fachbereich Physik, Universität Osnabrück, Barbarastr. 7, 49069 Osnabrück, Germany
M.-C. Schürmann: Fachbereich Physik, Universität Osnabrück, Barbarastr. 7, 49069 Osnabrück, Germany
S. Kühl: Fachbereich Physik, Universität Osnabrück, Barbarastr. 7, 49069 Osnabrück, Germany
M. Klusmann: Fachbereich Physik, Universität Osnabrück, Barbarastr. 7, 49069 Osnabrück, Germany
E. Rühl: Fachbereich Physik, Universität Osnabrück, Barbarastr. 7, 49069 Osnabrück, Germany

Surface Review and Letters (SRL), 2002, vol. 09, issue 01, 105-110

Abstract: The single-photon ionization mass spectrometry of primary photofragments of chlorine monoxide (ClO) is reported. The use of laser-produced plasma (LPP) radiation in pump–probe experiments allows us to ionize the laser-generated atomic photoproducts with tunable radiation in the vacuum ultraviolet regime (E = 10–18eV). Autoionization resonances of the atomic photoproducts are used to establish the quantum states of the photoproducts and to enhance the detection sensitivity. Predissociation and direct dissociation ofA(2Π)-excited ClO yieldsCl(2P)+O(3P)as well asCl(2P)+O(1D), respectively. The quantum yield ofO(1D)formation is reported in the threshold regime near the ClO[A(2Π)]dissociation limit.

Date: 2002
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DOI: 10.1142/S0218625X02002129

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