PHOTOELECTRONIC INVESTIGATION OFPdELECTRON STRUCTURE TRANSFORMATION AT OXYGEN ADSORPTION

V. P. Belash, I. N. Klimova and Yu. S. Mitrokhin
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V. P. Belash: Physical-Technical Institute, Ural Branch, Russian Academy of Sciences, Izhevsk, Udmurt Republic 426008, Russia
I. N. Klimova: Physical-Technical Institute, Ural Branch, Russian Academy of Sciences, Izhevsk, Udmurt Republic 426008, Russia
Yu. S. Mitrokhin: Department of Mathematics, Udmurt State University, Izhevsk, Udmurt Republic 426034, Russia

Surface Review and Letters (SRL), 2005, vol. 12, issue 05n06, 713-719

Abstract: Oxygen adsorption on the surface of polycrystalline palladium has been studied by the photoelectron spectroscopy method in a wide range of oxygen exposure and temperatures, starting with the earliest stages of adsorption to the formation of the surface compound ofPdO-type. Based on the analysis of the experimental data and the calculation of the density of states carried out by the TB-LMTO-ASA method, the attempt to elucidate the electronic mechanism of adsorption and oxidation power of palladium was made.

Keywords: Photoelectron spectra; adsorption; electronic structure; Fermi level (search for similar items in EconPapers)
Date: 2005
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DOI: 10.1142/S0218625X05007980

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