Iron oxide looping for natural gas conversion in a countercurrent moving bed reactor

Liang Zeng, Andrew Tong, Mandar Kathe, Samuel Bayham and Liang-Shih Fan

Applied Energy, 2015, vol. 157, issue C, 338-347

Abstract: Chemical looping technologies have the potential to reduce the natural-gas conversion cost in a carbon-constrained scenario. Given the increasing importance of natural gas to global energy supply, this work investigates the application of an iron oxide based chemical looping technology for natural gas conversion. A thermodynamic criterion for selecting iron oxide based oxygen carrier material and designing the reaction system is developed using an adapted Ellingham diagram. Equilibrium modeling for detailed thermodynamic analysis is conducted for verifying the Ellingham diagram analysis. The thermodynamic equilibrium model also establishes a system baseline performance, and experimental proof of concept bench-scale demonstration is investigated. The bench-scale testing is used to characterize the effect of parameters like solids to gas ratio and temperature of the reactor on system performance. An optimal set of operating conditions is identified for further testing on a larger scale.

Keywords: Chemical looping combustion; Oxygen carrier; Natural gas; Energy conversion; Carbon capture (search for similar items in EconPapers)
Date: 2015
References: View references in EconPapers View complete reference list from CitEc
Citations: View citations in EconPapers (7)

Downloads: (external link)
http://www.sciencedirect.com/science/article/pii/S0306261915007874
Full text for ScienceDirect subscribers only

Related works:
This item may be available elsewhere in EconPapers: Search for items with the same title.

Export reference: BibTeX RIS (EndNote, ProCite, RefMan) HTML/Text

Persistent link: https://EconPapers.repec.org/RePEc:eee:appene:v:157:y:2015:i:c:p:338-347

Ordering information: This journal article can be ordered from
http://www.elsevier.com/wps/find/journaldescription.cws_home/405891/bibliographic
http://www.elsevier. ... 405891/bibliographic

DOI: 10.1016/j.apenergy.2015.06.029

Access Statistics for this article

Applied Energy is currently edited by J. Yan

More articles in Applied Energy from Elsevier
Bibliographic data for series maintained by Catherine Liu ().